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author：

Sun, D. (Sun, D..) [1] | Fu, Y. (Fu, Y..) [2] | Liu, W. (Liu, W..) [3] | Ye, L. (Ye, L..) [4] | Wang, D. (Wang, D..) [5] | Yang, L. (Yang, L..) [6] | Fu, X. (Fu, X..) [7] | Li, Z. (Li, Z..) [8]

Indexed by：

Scopus

Abstract：

Metal-organic　framework　(MOF)　NH2-Uio-66(Zr)　exhibits　pho-tocatalytic　activity　for　CO2　reduction　in　the　presence　of　triethanolamine　as　sacrificial　agent　under　visible-light　irradiation.　Photoinduced　electron　transfer　from　the　excited　2-aminoterephthalate　(ATA)　to　Zr　oxo　clusters　in　NH2-Uio-66(Zr)　was　for　the　first　time　revealed　by　photoluminescence　studies.　Generation　of　ZrIII　and　its　involvement　in　photocatalytic　CO2　reduction　was　confirmed　by　ESR　analysis.　Moreover,　NH2-Uio-66(Zr)　with　mixed　ATA　and　2,　5-diaminoterephthalate　(DTA)　li-gands　was　prepared　and　shown　to　exhibit　higher　performance　for　photocatalytic　CO2　reduction　due　to　its　enhanced　light　adsorption　and　increased　adsorption　of　CO2.　This　study　provides　a　better　understanding　of　photocatalyt-ic　CO2　reduction　over　MOF-based　photocatalysts　and　also　demonstrates　the　great　potential　of　using　MOFs　as　highly　stable,　molecularly　tunable,　and　recyclable　photocatalysts　in　CO2　reduction.　©　2013　Wiley-VCH　Verlag　GmbH　&　Co.　KGaA.

Keyword：

Carbon dioxide fixation; Metal-organic frameworks; Photochemistry; Reduction; Zirconium

Community：

  • [ 1 ] [Sun, D.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China
  • [ 2 ] [Fu, Y.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China
  • [ 3 ] [Liu, W.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China
  • [ 4 ] [Ye, L.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China
  • [ 5 ] [Wang, D.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China
  • [ 6 ] [Yang, L.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China
  • [ 7 ] [Fu, X.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China
  • [ 8 ] [Li, Z.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China

Reprint 's Address：

  • [Li, Z.]Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou 350002, China

Email：


zhaohuili1969@yahoo.com
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Source ：

Chemistry - A European Journal

ISSN： 0947-6539

Year： 2013

Issue： 42

Volume： 19

Page： 14279-14285

5 . 6 9 6

JCR@2013

3 . 9 0 0

JCR@2023

JCR Journal Grade：1

CAS Journal Grade：2

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 566

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 3

Affiliated Colleges：

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