Synthesis of Layered Carbonitrides from Biotic Molecules for Photoredox Transformations - Details

author：

Yang, C. (Yang, C..) ^[1] | Wang, B. (Wang, B..) ^[2] | Zhang, L. (Zhang, L..) ^[3] | Yin, L. (Yin, L..) ^[4] | Wang, X. (Wang, X..) ^[5]

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Abstract：

The　construction　of　layered　covalent　carbon　nitride　polymers　based　on　tri-s-triazine　units　has　been　achieved　by　using　nucleobases　(adenine,　guanine,　cytosine,　thymine　and　uracil)　and　urea　to　establish　a　two-dimensional　semiconducting　structure　that　allows　band-gap　engineering　applications.　This　biomolecule-derived　binary　carbon　nitride　polymer　enables　the　generation　of　energized　charge　carrier　with　light-irradiation　to　induce　photoredox　reactions　for　stable　hydrogen　production　and　heterogeneous　organosynthesis　of　C−O,　C−C,　C−N　and　N−N　bonds,　which　may　enrich　discussion　on　chemical　reactions　in　prebiotic　conditions　by　taking　account　of　the　photoredox　function　of　conjugated　carbonitride　semiconductors　that　have　long　been　considered　to　be　stable　HCN-derived　organic　macromolecules　in　space.　©　2017　Wiley-VCH　Verlag　GmbH　&　Co.　KGaA,　Weinheim

Keyword：

carbon nitride semiconductors; chemical evolution; nucleobases; photocatalysis; urea

Community：

[ 1 ] [Yang, C.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350002, China
[ 2 ] [Wang, B.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350002, China
[ 3 ] [Zhang, L.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350002, China
[ 4 ] [Yin, L.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350002, China
[ 5 ] [Wang, X.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350002, China

Reprint 's Address：

[Wang, X.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou UniversityChina

Email：

xcwang@fzu.edu.cn

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Source ：

Angewandte Chemie - International Edition

ISSN： 1433-7851

Year： 2017

Issue： 23

Volume： 56

Page： 6627-6631

1 2 . 1 0 2

JCR@2017

1 6 . 1 0 0

JCR@2023

ESI HC Threshold：226

JCR Journal Grade：1

CAS Journal Grade：2

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 190

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 0

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