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author：

Ye, J. (Ye, J..) [1] | Wu, J. (Wu, J..) [2] | Lv, T. (Lv, T..) [3] | Wu, G. (Wu, G..) [4] | Gao, Y. (Gao, Y..) [5] | Chen, H. (Chen, H..) [6]

Indexed by：

Scopus

Abstract：

The　observation　of　an　unexpected　oxidative　rearrangement　coupling　reaction　led　to　the　development　of　a　novel　method　for　the　efficient　functionalization　of　tetrahydro-β-carbolines　(THβCs).　The　treatment　of　THβCs　with　photogenerated　singlet　oxygen　(　1　O　2　)　afforded　unstable　dioxetanes,　which　underwent　further　transformation　to　form　new　bonds　in　the　presence　of　trifluoroacetic　acid.　This　operationally　simple　protocol　exhibits　broad　functional-group　tolerance　and　is　suitable　for　the　late-stage　functionalization　of　complex　druglike　molecules.　©　2017　Wiley-VCH　Verlag　GmbH　&　Co.　KGaA,　Weinheim.

Keyword：

oxidative functionalization; rearrangement; singlet oxygen; tetrahydro-β-carbolines; visible light

Community：

  • [ 1 ] [Ye, J.]College of Chemistry, Fuzhou University, Fuzhou, Fujian 350116, China
  • [ 2 ] [Wu, J.]College of Chemistry, Fuzhou University, Fuzhou, Fujian 350116, China
  • [ 3 ] [Lv, T.]College of Chemistry, Fuzhou University, Fuzhou, Fujian 350116, China
  • [ 4 ] [Wu, G.]College of Chemistry, Fuzhou University, Fuzhou, Fujian 350116, China
  • [ 5 ] [Gao, Y.]College of Chemistry, Fuzhou University, Fuzhou, Fujian 350116, China
  • [ 6 ] [Chen, H.]College of Chemistry, Fuzhou University, Fuzhou, Fujian 350116, China

Reprint 's Address：

  • [Chen, H.]College of Chemistry, Fuzhou UniversityChina

Email：


chenhaij@gmail.com
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Source ：

Angewandte Chemie - International Edition

ISSN： 1433-7851

Year： 2017

Issue： 47

Volume： 56

Page： 14968-14972

1 2 . 1 0 2

JCR@2017

1 6 . 1 0 0

JCR@2023

ESI HC Threshold：226

JCR Journal Grade：1

CAS Journal Grade：2

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 41

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 0

Affiliated Colleges：

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