Robust Photocatalytic H2O2 Production by Octahedral Cd3(C3N3S3)2 Coordination Polymer under Visible Light - Details

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Abstract：

Herein,　we　reported　a　octahedral　Cd3(C3N3S3)2　coordination　polymer　as　a　new　noble　metal-free　photocatalyst　for　robust　photocatalytic　H2O2　production　from　methanol/water　solution.　The　coordination　polymer　can　give　an　unprecedented　H2O2　yield　of　ca.　110.0mmol•L-1•g-1　at　pH=2.8　under　visible　light　illumination.　The　characterization　results　clearly　revealed　that　the　photocatalytic　H2O2　production　proceeds　by　a　pathway　of　two-electron　reduction　of　O2　on　the　catalyst　surface.　This　work　showed　the　potential　perspective　of　Mx(C3N3S3)y　(M=transitional　metals)　coordination　polymers　as　a　series　of　new　materials　for　solar　energy　storage　and　conversion.　©　2015,　Nature　Publishing　Group.　All　rights　reserved.

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[ 1 ] [Zhuang, H.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 2 ] [Yang, L.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 3 ] [Xu, J.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 4 ] [Li, F.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 5 ] [Zhang, Z.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 6 ] [Lin, H.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 7 ] [Long, J.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 8 ] [Wang, X.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China

Reprint 's Address：

[Long, J.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou UniversityChina

Email：

jllong@fzu.edu.cn

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Scientific Reports

ISSN： 2045-2322

Year： 2015

Volume： 5

5 . 2 2 8

JCR@2015

3 . 8 0 0

JCR@2023

ESI HC Threshold：500

JCR Journal Grade：1

CAS Journal Grade：2

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WoS CC Cited Count：

SCOPUS Cited Count： 75

ESI Highly Cited Papers on the List： 0 Unfold All

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Chinese Cited Count：

30 Days PV： 1

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