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author:

He, Y. (He, Y..) [1] | Zhang, L.M. (Zhang, L.M..) [2] | Chen, Y.M. (Chen, Y.M..) [3] | Sun, L. (Sun, L..) [4] | Hu, C. (Hu, C..) [5] | Wang, M.X. (Wang, M.X..) [6] | Gao, Y. (Gao, Y..) [7] | Yang, J.H. (Yang, J.H..) [8] | Zhang, Q.Q. (Zhang, Q.Q..) [9]

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Scopus

Abstract:

Exploring photoluminescent silk fibers, possessing biocompatibility as well as stable and durable fluorescent properties, is a requirement for the development of novel photoluminescent biomaterials. Herein, we fabricate photoluminescent silk fibers, TPCA@SF, via modifying an organic fluorescent molecule (5-oxo-3,5-dihydro-2H-thiazolo [3,2-a] pyridine-7-carboxylic acid, TPCA) onto silk fibers, along with using quaternary ammonium salt didodecyldimethylammonium bromide (DDAB) as a color-fixing agent. The hydrogen bonds and electrostatic association among silk fibers, TPCA and DDAB, ensure the stable modification. The facile and green fabrication process is achieved in water under mild conditions without using any toxic substances. The TPCA@SF manifests the combining features of high quantum yield, fluorescence water-fastness, antiphotobleaching, good mechanical property, and biocompatibility. The strategy holds great potential for exploring various biocompatible photoluminescent substances with stability and durability. © 2019 American Chemical Society.

Keyword:

antiphotobleaching; biocompatibility; photoluminescence; silk fibers; wash-durability

Community:

  • [ 1 ] [He, Y.]State Key Laboratory for Strength and Vibration of Mechanical Structures, International Center for Applied Mechanics, School of Aerospace Engineering, Collaborative Innovation Center of Suzhou Nano Science and Technology, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 2 ] [Zhang, L.M.]State Key Laboratory for Strength and Vibration of Mechanical Structures, International Center for Applied Mechanics, School of Aerospace Engineering, Collaborative Innovation Center of Suzhou Nano Science and Technology, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 3 ] [Chen, Y.M.]State Key Laboratory for Strength and Vibration of Mechanical Structures, International Center for Applied Mechanics, School of Aerospace Engineering, Collaborative Innovation Center of Suzhou Nano Science and Technology, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 4 ] [Chen, Y.M.]College of Bioresources Chemical and Materials Engineering, Shaanxi University of Science and Technology, Key Laboratory of Leather Cleaner Production, China National Light Industry, Xi'an, Shaanxi, 710021, China
  • [ 5 ] [Sun, L.]School of Science, State Key Laboratory for Mechanical Behaviour of Materials, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 6 ] [Hu, C.]School of Science, State Key Laboratory for Mechanical Behaviour of Materials, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 7 ] [Wang, M.X.]School of Science, State Key Laboratory for Mechanical Behaviour of Materials, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 8 ] [Gao, Y.]State Key Laboratory for Strength and Vibration of Mechanical Structures, International Center for Applied Mechanics, School of Aerospace Engineering, Collaborative Innovation Center of Suzhou Nano Science and Technology, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 9 ] [Yang, J.H.]State Key Laboratory for Strength and Vibration of Mechanical Structures, International Center for Applied Mechanics, School of Aerospace Engineering, Collaborative Innovation Center of Suzhou Nano Science and Technology, Xi'An Jiaotong University, Xi'an, Shaanxi, 710049, China
  • [ 10 ] [Zhang, Q.Q.]Institute of Biomedical and Pharmaceutical Technology, Fuzhou University, Fuzhou, Fujian, 350002, China
  • [ 11 ] [Zhang, Q.Q.]Fujian Guided Tissue Regeneration (GTR) Biotechnology Co., Ltd., Fuzhou, 350108, China

Reprint 's Address:

  • [Chen, Y.M.]State Key Laboratory for Strength and Vibration of Mechanical Structures, International Center for Applied Mechanics, School of Aerospace Engineering, Collaborative Innovation Center of Suzhou Nano Science and Technology, Xi'An Jiaotong UniversityChina

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Source :

ACS Biomaterials Science and Engineering

ISSN: 2373-9878

Year: 2019

Issue: 5

Volume: 5

Page: 2657-2668

4 . 1 5 2

JCR@2019

5 . 5 0 0

JCR@2023

ESI HC Threshold:236

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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