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author:

Zhang, Z. (Zhang, Z..) [1] | Huang, L. (Huang, L..) [2] | Zhang, J. (Zhang, J..) [3] | Wang, F. (Wang, F..) [4] | Xie, Y. (Xie, Y..) [5] | Shang, X. (Shang, X..) [6] | Gu, Y. (Gu, Y..) [7] | Zhao, H. (Zhao, H..) [8] | Wang, X. (Wang, X..) [9]

Indexed by:

Scopus

Abstract:

Construction of heterostructure by intimately interfacing two or more semiconductor materials with different geometrical and electronically energetic alignments at nanoscale is very important to achieve the composite photocatalysts with a high photocatalytic efficiency. Here, we in-situ prepared an intimate contact MoS2/ZnIn2S4 heterostructure photocatalyst by a one-pot solvothermal reaction. The MoS2/ZnIn2S4 heterostructure significantly enhanced the photocatalytic H2 evolution of ZnIn2S4 under visible light illumination. The hydrogen evolution rate reaches 3891.6 μmol g−1 h−1 over 5%-MoS2/ZnIn2S4, which exceeded the photocatalytic activity of Pt-loaded ZnIn2S4 samples. The subtle atomic-level intimate contact and strong interactions between ZnIn2S4 and MoS2 was ascribed to a highly efficient charge carrier separation and thus photocatalytic activity for MoS2/ZnIn2S4. These results provide inspiration for the design of composited photocatalysts with efficient photocatalytic H2 evolution. © 2018 Elsevier B.V.

Keyword:

H2 evolution; Heterostructure; MoS2/ZnIn2S4; Photocatalysis

Community:

  • [ 1 ] [Zhang, Z.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 2 ] [Huang, L.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 3 ] [Zhang, J.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 4 ] [Wang, F.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 5 ] [Xie, Y.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 6 ] [Shang, X.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 7 ] [Gu, Y.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 8 ] [Zhao, H.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China
  • [ 9 ] [Wang, X.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou University, China

Reprint 's Address:

  • [Zhang, Z.]State Key Laboratory of Photocatalysis on Energy and Environment, Research Institute of Photocatalysis, College of Chemistry, Fuzhou UniversityChina

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Source :

Applied Catalysis B: Environmental

ISSN: 0926-3373

Year: 2018

Volume: 233

Page: 112-119

1 4 . 2 2 9

JCR@2018

2 0 . 3 0 0

JCR@2023

ESI HC Threshold:209

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 199

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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