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author:

Li, Peipei (Li, Peipei.) [1] | Schott, Jennifer A. (Schott, Jennifer A..) [2] | Zhang, Jinshui (Zhang, Jinshui.) [3] | Mahurin, Shannon M. (Mahurin, Shannon M..) [4] | Sheng, Yujie (Sheng, Yujie.) [5] | Qiao, Zhen-An (Qiao, Zhen-An.) [6] | Hu, Xunxiang (Hu, Xunxiang.) [7] | Cui, Guokai (Cui, Guokai.) [8] | Yao, Dongdong (Yao, Dongdong.) [9] | Brown, Suree (Brown, Suree.) [10] | Zheng, Yaping (Zheng, Yaping.) [11] | Dai, Sheng (Dai, Sheng.) [12]

Indexed by:

EI

Abstract:

Porous liquids are a newly developed porous material that combine unique fluidity with permanent porosity, which exhibit promising functionalities for a variety of applications. However, the apparent incompatibility between fluidity and permanent porosity makes the stabilization of porous nanoparticle with still empty pores in the dense liquid phase a significant challenging. Herein, by exploiting the electrostatic interaction between carbon networks and polymerized ionic liquids, we demonstrate that carbon-based porous nanoarchitectures can be well stabilized in liquids to afford permanent porosity, and thus opens up a new approach to prepare porous carbon liquids. Furthermore, we hope this facile synthesis strategy can be widely applicated to fabricate other types of porous liquids, such as those (e.g., carbon nitride, boron nitride, metal–organic frameworks, covalent organic frameworks etc.) also having the electrostatic interaction with polymerized ionic liquids, evidently advancing the development and understanding of porous liquids. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Keyword:

Carbon nitride Coulomb interactions Electrostatics Electrostatic separators Fluidity III-V semiconductors Ionic liquids Nitrides Polymers Porosity Porous materials

Community:

  • [ 1 ] [Li, Peipei]Chemical Science Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 2 ] [Li, Peipei]Key Laboratory of Space Applied Physics and Chemistry, Ministry of Education, School of Natural and Applied Sciences, Northwestern Polytechnical University, Xi'an; Shaanxi; 710129, China
  • [ 3 ] [Schott, Jennifer A.]Chemical Science Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 4 ] [Schott, Jennifer A.]Department of Chemistry, University of Tennessee, Knoxville; TN; 37996, United States
  • [ 5 ] [Zhang, Jinshui]Chemical Science Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 6 ] [Zhang, Jinshui]State Key Laboratory of Photocatalysis on Energy and Environment; College of Chemistry, Fuzhou University, Fouzhou; 350116, China
  • [ 7 ] [Mahurin, Shannon M.]Chemical Science Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 8 ] [Sheng, Yujie]Chemical Science Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 9 ] [Qiao, Zhen-An]State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, International Joint Research Laboratory of Nano-Micro Architecture Chemistry, College of Chemistry, Jilin University, Changchun; Jilin; 130012, China
  • [ 10 ] [Hu, Xunxiang]Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 11 ] [Cui, Guokai]Chemical Science Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 12 ] [Yao, Dongdong]Key Laboratory of Space Applied Physics and Chemistry, Ministry of Education, School of Natural and Applied Sciences, Northwestern Polytechnical University, Xi'an; Shaanxi; 710129, China
  • [ 13 ] [Brown, Suree]Department of Chemistry, University of Tennessee, Knoxville; TN; 37996, United States
  • [ 14 ] [Zheng, Yaping]Key Laboratory of Space Applied Physics and Chemistry, Ministry of Education, School of Natural and Applied Sciences, Northwestern Polytechnical University, Xi'an; Shaanxi; 710129, China
  • [ 15 ] [Dai, Sheng]Chemical Science Division, Oak Ridge National Laboratory, Oak Ridge; TN; 37831, United States
  • [ 16 ] [Dai, Sheng]Department of Chemistry, University of Tennessee, Knoxville; TN; 37996, United States

Reprint 's Address:

  • [zhang, jinshui]chemical science division, oak ridge national laboratory, oak ridge; tn; 37831, united states;;[zhang, jinshui]state key laboratory of photocatalysis on energy and environment; college of chemistry, fuzhou university, fouzhou; 350116, china

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Source :

Angewandte Chemie - International Edition

ISSN: 1433-7851

Year: 2017

Issue: 47

Volume: 56

Page: 14958-14962

1 2 . 1 0 2

JCR@2017

1 6 . 1 0 0

JCR@2023

ESI HC Threshold:226

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 66

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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