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author:

Hu, Xiang (Hu, Xiang.) [1] | Liu, Yangjie (Liu, Yangjie.) [2] | Chen, Junxiang (Chen, Junxiang.) [3] | Jia, Jingchun (Jia, Jingchun.) [4] | Zhan, Hongbing (Zhan, Hongbing.) [5] (Scholars:詹红兵) | Wen, Zhenhai (Wen, Zhenhai.) [6]

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EI Scopus SCIE

Abstract:

Sodium-ion hybrid capacitors (SIHCs) have shown great promise in achieving both high energy density and high power density by virtue of synergizing the merits of batteries and capacitors. However, the lack of favorable anode material with superior sodium-ion storage capability is still a major challenge in the development of high-performance SIHCs. Herein, we report the design and synthesis of a promising sodium-ion storage nanohybrid with FeS quantum dots embedded in three-dimensional (3D) inverse opal (IO)-structured N-doped carbon (3D-IO FeS-QDs@NC). By virtue of the robust 3D conductive architecture, the 3D-IO FeS-QDs@NC nanohybrid exhibits favorable features of excellent electron/ion transport kinetics, superior structural stability, as well as impressive sodium-ion storage capability with high specific capacity, outstanding rate capability, and ultra-long cyclic stability. Such highly desirable sodium storage performance inspired us to study their potential application in SHICs by coupling with commercial activated carbon (AC) as a cathode. The as-developed SHICs can deliver a maximum energy density and power output of 151.8 W h kg(-1) and 9280 W kg(-1), respectively, and an excellent cycling lifespan with 91% capacity retention after 5000 cycles at 1 A g(-1), which holds promise for bridging the performance gap between conventional batteries and capacitors.

Keyword:

Community:

  • [ 1 ] [Hu, Xiang]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 2 ] [Liu, Yangjie]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 3 ] [Zhan, Hongbing]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 4 ] [Hu, Xiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350116, Fujian, Peoples R China
  • [ 5 ] [Liu, Yangjie]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350116, Fujian, Peoples R China
  • [ 6 ] [Chen, Junxiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350116, Fujian, Peoples R China
  • [ 7 ] [Jia, Jingchun]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350116, Fujian, Peoples R China
  • [ 8 ] [Wen, Zhenhai]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350116, Fujian, Peoples R China

Reprint 's Address:

  • 詹红兵

    [Zhan, Hongbing]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China;;[Wen, Zhenhai]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350116, Fujian, Peoples R China

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Source :

JOURNAL OF MATERIALS CHEMISTRY A

ISSN: 2050-7488

Year: 2019

Issue: 3

Volume: 7

Page: 1138-1148

1 1 . 3 0 1

JCR@2019

1 0 . 8 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:236

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 101

SCOPUS Cited Count: 105

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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